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Anthocyanins/chitosan films doped by nano zinc oxide for active and intelligent packaging: comparison

《化学科学与工程前沿（英文）》 2023年第17卷第6期页码 704-715 doi: 10.1007/s11705-022-2270-z

摘要： The multifunctional films was prepared by blending chitosan and nano-ZnO with purple tomato anthocyanins or black wolfberry anthocyanins. The properties of films functioned by anthocyanins source and nano-ZnO content were studied. It was found purple tomato anthocyanins showed more significant color change against pH than black wolfberry anthocyanins. The nano-ZnO were widely dispersed in matrix and enhanced the compatibility of anthocyanins with chitosan. However, the anthocyanins source influenced the properties of the films more slightly than nano-ZnO addition. The tensile strength, antioxidant and antibacterial effects of the chitosan films dramatically increased after cooperated by nano-ZnO and anthocyanins, which also enhanced with increase of nano-ZnO content, whereas the elongation at break of the composite films decreased. Especially, the anthocyanin and nano-ZnO promoted the antibacterial activity of films synergistically. Composite films made from black wolfberry anthocyanins exhibited higher mechanical performance than those made from purple tomato anthocyanins but weaker antibacterial effects. The purple tomato anthocyanins/chitosan and nano-ZnO/purple tomato anthocyanins/chitosan films effectively reflected pork spoilage, changing their colors from dark green to brown, indicating the potential for applications in active and intelligent food packaging.

关键词： bio-based multifunction colorimetric indicator active and intelligent packaging

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ENVIRONMENTAL ATTITUDES AND CONSUMER PREFERENCE FOR ENVIRONMENTALLY-FRIENDLY BEVERAGE PACKAGING: THE

《农业科学与工程前沿（英文）》 2023年第10卷第1期页码 95-108 doi: 10.15302/J-FASE-2022478

摘要：

● Consumer preference for environmentally-friendly beverage packaging was investigated.

关键词： China consumer preference food and beverage packaging green identity label information treatment plastics

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Thermal and catalytic pyrolysis of a synthetic mixture representative of packaging plastics residue

Simona Colantonio, Lorenzo Cafiero, Doina De Angelis, Nicolò M. Ippolito, Riccardo Tuffi, Stefano Vecchio Ciprioti

《化学科学与工程前沿（英文）》 2020年第14卷第2期页码 288-303 doi: 10.1007/s11705-019-1875-3

摘要： A synthetic mixture of real waste packaging plastics representative of the residue from a material recovery facility (plasmix) was submitted to thermal and catalytic pyrolysis. Preliminary thermogravimetry experiments coupled with Fourier transform infrared spectroscopy were performed to evaluate the effects of the catalysts on the polymers’ degradation temperatures and to determine the main compounds produced during pyrolysis. The thermal and catalytic experiments were conducted at 370°C, 450°C and 650°C using a bench scale reactor. The oil, gas, and char yields were analyzed and the compositions of the reaction products were compared. The primary aim of this study was to understand the effects of zeolitic hydrogen ultra stable zeolite Y (HUSY) and hydrogen zeolite socony mobil-5 (HZSM5) catalysts with high silica content on the pyrolysis process and the products’ quality. Thermogravimetry showed that HUSY significantly reduces the degradation temperature of all the polymers—particularly the polyolefines. HZSM5 had a significant effect on the degradation of polyethylene due to its smaller pore size. Mass balance showed that oil is always the main product of pyrolysis, regardless of the process conditions. However, all pyrolysis runs performed at 370°C were incomplete. The use of either zeolites resulted in a decrease in the heavy oil fraction and the prevention of wax formation. HUSY has the best performance in terms of the total monoaromatic yield (29 wt-% at 450°C), while HZSM5 promoted the production of gases (41 wt-% at 650°C). Plasmix is a potential input material for pyrolysis that is positively affected by the presence of the two tested zeolites. A more effective separation of polyethylene terephthalate during the selection process could lead to higher quality pyrolysis products.

关键词： packaging plastics waste plasmix pyrolysis zeolite catalyst degradation temperature

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Multi-Component Resource Recycling from Waste Light-Emitting Diode Under Hydrothermal Condition: Plastic Package Degradation, Speciation of Nano-TiO2, and Environmental Impact Assessment

Yongliang Zhang,Lu Zhan,Zhenming Xu,

《工程（英文）》 doi: 10.1016/j.eng.2023.04.008

摘要： Light emitting diodes (LEDs) have accounted for most of the lighting market as the technology matures and costs continue to reduce. As a new type of e-waste, LED is a double-edged sword, as it contains not only precious and rare metals but also organic packaging materials. In previous studies, LED recycling focused on recovering precious and strategic metals while ignoring harmful substances such as organic packaging materials. Unlike crushing and other traditional methods, hydrothermal treatment can provide an environment-friendly process for decomposing packaging materials. This work developed a closed reaction vessel, where the degradation rate of plastic polyphthalamide (PPA) was close to 100%, with nano-TiO₂ encapsulated in plastic PPA being efficiently recovered, while metals contained in LED were also recycled efficiently. Besides, the role of water in plastic PPA degradation that has been overlooked in current studies was explored and speculated in detail in this work. Environmental impact assessment revealed that the proposed recycling route for waste LED could significantly reduce the overall environmental impact compared to the currently published processes. Especially the developed method could reduce more than half the impact of global warming. Furthermore, this research provides a theoretical basis and a promising method for recycling other plastic-packaged e-waste devices, such as integrated circuits.

关键词： Waste LED Hydrothermal treatment Recycling Plastic PPA degradation Packaging materials

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用于微电子机械系统封装的体硅键合技术和薄膜密封技术

王渭源,王跃林

《中国工程科学》 2002年第4卷第6期页码 56-62

摘要：

对静电键合、体硅直接键合和界面层辅助键合等三种体硅键合技术，整片操作、局部操作和选择保护等三种密封技术，以及这些技术用于微电子机械系统的密封作了评述，强调在器件研究开始时应考虑封装问题，具体技术则应在保证器件功能和尽量减少芯片复杂性两者之间权衡决定。

关键词：体硅键合技术薄膜密封技术微电子机械系统封装技术

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基于玻璃通孔的Ka波段宽带滤波封装天线 Research Article

方针1,2,张继华1,2,3,高莉彬1,2,陈宏伟1,2,李文磊1,2,梁天鹏1,2,蔡旭东1,2,蔡星周3,贾惟聪3,郭欢3,李勇3

《信息与电子工程前沿（英文）》 2023年第24卷第6期页码 916-926 doi: 10.1631/FITEE.2200573

摘要：以玻璃封装材料和玻璃通孔技术为基础，提出一种新的Ka波段(33 GHz)滤波封装天线(FPA)，该天线具有宽频带和高滤波响应特点。与传统封装材料(印刷电路板、低温共烧陶瓷、硅等)相比，玻璃通孔更适合小型化技术(毫米波三维封装器件)，具有优越的微波性能。玻璃基板通过键合技术可实现三维高密度互联，其热膨胀系数与硅相当。此外，玻璃基板的堆叠实现了高密度互连，并与微电子技术兼容。该天线辐射贴片由贴片天线和反射系数几乎互补的带通滤波器(BPF)组成。BPF单元有3对λg/4槽(缺陷微带结构)和两对λg/2 U形缝隙(缺陷地结构)。该天线实现了大带宽和高辐射效率，这可能与玻璃基板的叠加和玻璃通孔馈电有关。此外，引入4个辐射零值可有效提高阻带内的抑制水平。为验证所提设计性能，对33 GHz宽带滤波天线进行优化、调试和测量。天线的工作带宽为29.4‒36.4 GHz (|S11|<−10 dB)，阻抗匹配带宽高达21.2%，阻带抑制水平大于16.5 dB。该天线实际增益为~6.5 dBi，辐射效率为~89%。

关键词：滤波封装天线；玻璃通孔；三维封装器件；激光键合

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The road to sustainable use and waste management of plastics in Portugal

《环境科学与工程前沿（英文）》 2022年第16卷第1期页码 5-5 doi: 10.1007/s11783-021-1439-x

摘要：

• Portugal recycles 34% of the 40 kg/hab year of plastic packaging waste.

关键词： Single-use plastics Plastic packaging Plastic waste Waste management Waste shipment Lightweight plastic bags

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The electrostatic-alloy bonding technique used in MEMS

WANG Wei, CHEN Wei-ping

《机械工程前沿（英文）》 2006年第1卷第2期页码 238-241 doi: 10.1007/s11465-006-0011-5

摘要： Electrostatic-alloy bonding of silicon wafer with glass deposited by Au to form Si/Au-glass water, and bonding of Si/Au-glass with silicon wafer were researched during fabrication of pressure sensors. The silicon wafer and glass wafer with an Au film resistor were bonded by electrostatic bonding, and then Si-Au alloy bonding was formed by annealing at 400vH for 2 h. The air sealability of the cavity after bonding was finally tested using the N filling method. The results indicate that large bond strength was obtained at the bonding interface. This process was used in fabricating a pressure sensor with a sandwich structure. The results indicate that the sensor presented better performances and that the bonding techniques can be used in MEMS packaging.

关键词： Si/Au-glass strength MEMS packaging process sandwich structure

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Hierarchically porous zeolites synthesized with carbon materials as templates

《化学科学与工程前沿（英文）》 2021年第15卷第6期页码 1444-1461 doi: 10.1007/s11705-021-2090-6

摘要： Hierarchically porous zeolites are promising candidates in catalytic conversion of relatively bulky molecules, and their syntheses have attracted significant attention. From both industrial and scientific perspectives, different carbon materials have been widely employed as hard templates for the preparation of hierarchically porous zeolites during the past two decades. In this review, the progress in synthetic strategies using carbon materials as templates is comprehensively summarized. Depending on the affinity between the carbon templates and zeolite precursors, the substantial strategies for synthesizing hierarchical zeolites are introduced in direct templates and indirect templates. Direct templates methods, by which the carbon materials are directly mixed with precursors gel as hard templates, are first reviewed. Then, we discuss the indirect templates method (crystallization of carbon-silica composites), by which the carbon is produced by in situ pyrolysis of organic-inorganic precursors. In addition, the technique of encapsulating metal species into zeolites crystals with the assistance of carbon templates is also discussed. In the conclusion part, the factors affecting the synthesis of carbon-templated hierarchically porous zeolites are remarked. This review is expected to attract interest in the synthesis strategies of hierarchically porous zeolites, especially cost-effective and large-scale production methodologies, which are essential to the industrial application of hierarchical zeolites.

关键词： hierarchical zeolites carbon materials direct templates indirect templates carbon-silica composites

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Influence of envelope insulation materials on building energy consumption

Junlan YANG, Jiabao TANG

《能源前沿（英文）》 2017年第11卷第4期页码 575-581 doi: 10.1007/s11708-017-0473-7

摘要： In this paper, the influence of different external wall insulation materials on the energy consumption of a newly built apartment in Germany is investigated. Three types of insulation materials commonly used in Germany including mineral fiber, polyurethane, and vacuum insulation panel are chosen for the case studies. An energy analysis model is established to clarify the primary energy use for production of the insulation materials and for building space heating. The calculation results show that the energy consumption for insulation material production increases with the insulation thickness, whereas the energy use for space heating decreases with the insulation thickness. Thus, there exists an optimum thickness to get the lowest total energy consumption for each kind of insulation material. The ascending order of the total energy consumption of the three materials is mineral fiber, polyurethane, and vacuum insulation panel. However, the optimum insulation thicknesses for the three insulation materials show a verse order at a certain heat transfer coefficient of the base envelope. The energy payback time (EPT) is proposed to calculate the payback time of the primary energy use for insulation material production. Mineral fiber has the shortest time, followed by polyurethane and vacuum insulation panel. The EPTS is 10, 19 and 21 years, respectively when the heat transfer coefficient of the base envelope is 0.2 W/(m ·K). In addition, the simulated results show that the theoretical value and the simulated value are basically identical.

关键词： building envelope insulation materials energy consumption payback time

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Emerging electrochemical processes for materials recovery from wastewater: Mechanisms and prospects

Lingchen Kong, Xitong Liu

《环境科学与工程前沿（英文）》 2020年第14卷第5期 doi: 10.1007/s11783-020-1269-2

摘要： Abstract • Mechanisms for selective recovery of materials in electrochemical processes are discussed. • Wastewaters that contain recoverable materials are reviewed. • Application prospects are discussed from both technical and non-technical aspects. Recovering valuable materials from waste streams is critical to the transition to a circular economy with reduced environmental damages caused by resource extraction activities. Municipal and industrial wastewaters contain a variety of materials, such as nutrients (nitrogen and phosphorus), lithium, and rare earth elements, which can be recovered as value-added products. Owing to their modularity, convenient operation and control, and the non-requirement of chemical dosage, electrochemical technologies offer a great promise for resource recovery in small-scale, decentralized systems. Here, we review three emerging electrochemical technologies for materials recovery applications: electrosorption based on carbonaceous and intercalation electrodes, electrochemical redox processes, and electrochemically induced precipitation. We highlight the mechanisms for achieving selective materials recovery in these processes. We also present an overview of the advantages and limitations of these technologies, as well as the key challenges that need to be overcome for their deployment in real-world systems to achieve cost-effective and sustainable materials recovery.

关键词： Materials recovery Electrosorption Capacitive deionization Redox processes Electrochemical precipitation

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Promoting hydrogen industry with high-capacity Mg-based solid-state hydrogen storage materials and systems

《能源前沿（英文）》 2023年第17卷第3期页码 320-323 doi: 10.1007/s11708-023-0889-1

摘要： Promoting hydrogen industry with high-capacity Mg-based solid-state hydrogen storage materials and systems

关键词： materials systems

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Advanced materials: adsorbent and catalyst for environmental application

Junhua LI, Shubo DENG

《环境科学与工程前沿（英文）》 2013年第7卷第3期页码 301-301 doi: 10.1007/s11783-013-0529-9

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Recycling Materials from Waste Electrical and Electronic Equipment

Jinhui Li

《环境科学与工程前沿（英文）》 2017年第11卷第5期 doi: 10.1007/s11783-017-1001-z

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Preface to special issue on “Advanced Materials and Catalysis”

《化学科学与工程前沿（英文）》 2021年第15卷第6期页码 1357-1359 doi: 10.1007/s11705-021-2119-x

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标题作者时间类型操作

Anthocyanins/chitosan films doped by nano zinc oxide for active and intelligent packaging: comparison

期刊论文

ENVIRONMENTAL ATTITUDES AND CONSUMER PREFERENCE FOR ENVIRONMENTALLY-FRIENDLY BEVERAGE PACKAGING: THE

期刊论文

Thermal and catalytic pyrolysis of a synthetic mixture representative of packaging plastics residue

Simona Colantonio, Lorenzo Cafiero, Doina De Angelis, Nicolò M. Ippolito, Riccardo Tuffi, Stefano Vecchio Ciprioti

期刊论文

Multi-Component Resource Recycling from Waste Light-Emitting Diode Under Hydrothermal Condition: Plastic Package Degradation, Speciation of Nano-TiO2, and Environmental Impact Assessment

Yongliang Zhang,Lu Zhan,Zhenming Xu,

期刊论文

用于微电子机械系统封装的体硅键合技术和薄膜密封技术

王渭源,王跃林

期刊论文

基于玻璃通孔的Ka波段宽带滤波封装天线

方针1,2,张继华1,2,3,高莉彬1,2,陈宏伟1,2,李文磊1,2,梁天鹏1,2,蔡旭东1,2,蔡星周3,贾惟聪3,郭欢3,李勇3

期刊论文

The road to sustainable use and waste management of plastics in Portugal

期刊论文

The electrostatic-alloy bonding technique used in MEMS

WANG Wei, CHEN Wei-ping